I'm on both Tuta and Proton, no clear winner but it depends on what you need as they are vastly different:
Proton is fast, pretty, compatible with Thunderbird and OpenPGP, very well integrated with proton pass and proton drive (e.g. you get email aliasing right inside your password manager). Proton doesn't give you reliable notifications on GrapheneOS without installing Sandboxes Play Services. They are also a bit behind Tuta when it comes to security and privacy implementations (privacy of notifications, quantum secure encryption etc). And it doesn't have feature parity beyond OSes.
Tuta is somewhat ugly, slow and incompatible with third party apps. But if you're willing to accept this, you get their own implementation of notifications (works without Play Services) and cutting edge security and privacy technology.
I'm slowly moving my setup (Bitwarden, Tresorit, Tuta, Mullvad) over to Proton Suite as it is more convenient. But if you prefer compartmentalization and the highest standards and are willing to compromise in speed and design, you should probably go with Tuta.
Both have a free plan, so maybe check them out and see whether one is fundamentally superior for your threat model and situation. Maybe you end up using both for different purposes even.